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Teacher of Chemistry Teacher of Chemical & Biomolecular Engineering 211 Lewis Hall (510) 642-0860 (510) 642-8369 209 Lewis (510) 643-3832 Research Study Expertise and Interest Inorganic and products chemistry; synthesis of inorganic particles and higher dimensional solids; exact tailoring of chemical and physical properties; gas storage, molecular separations, and catalysis in porous products; magnetic and conductive materials.

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We utilize a series of physical methods to evaluate and define our products comprehensively, consisting of by gas adsorption analysis, X-ray and neutron diffraction, different spectroscopic strategies, and SQUID magnetometry. For more details about the Long group and a complete list of publications, please go to the group website. Metal, Organic Frameworks A significant focus of research study in the Long group is the style and research study of metalorganic frameworksporous, inorganic solids developed of metal nodes linked by organic linkersthat are of interest for applications ranging from gas storage and molecular separations to catalysis and battery applications.

In addition, now more than ever global warming is demanding a dramatic decrease in our global greenhouse emissions. Among the most appealing short-term emissions mitigation strategiesand therefore a crucial separations needis the removal of CO2 directly from the flue gas streams of coal- and natural gas-fired power plants. Toward this end, we are studying a brand-new class of diamine-appended frameworks developed in our group that exhibit high CO2 separation capacities in the existence of water, with very little energy requirements developing from an unprecedented cooperative adsorption system.

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We are also targeting metalorganic structures including polarizing open metal sites and shape-discriminating pore structures for the boosted binding of H2 and CH4 near ambient temperatures and the separation of hydrocarbon isomers, respectively. The high-capacity storage of hydrogen and natural gas is particularly relevant for automotive transport, as these gases represent promising cleaner alternatives to liquid hydrocarbon fuels, and yet significant advances in adsorbent innovations are needed to get rid of the expensive constraints currently imposed by low-temperature and high-pressure on-board storage requirements.

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Catalysis and Conductivity In addition to their function as molecular screens, metalorganic structures are guaranteeing as robust, effective drivers with isolated and distinct active sites. We are seeking to utilize coordinatively-unsaturated structure metal centers as catalytic sites and also installing these metal focuses post-synthetically through chelating groups built into the framework ligands.